Publications

Towards predictive multidimensional modeling for industrializing microwave air plasma-based NOx formation

This publication presents a fluid model for (near-)atmospheric pressure air microwave plasma that couples fluid dynamics, microwave field heating, thermal chemistry, and the transport of chemically reactive species.
Authors: Matthias Albrechts, Ivan Tsonev, Vojtěch Laitl, Annemie Bogaerts

Removal of trace CH4 emissions by warm O2 plasma is kinetically limited: Insights from modeling and experiments

This publication investigates the potential of a warm O₂ plasma effluent for the removal of trace CH₄ concentrations in ambient air, using a combination of modeling and experiments.
Authors: Matthias Albrechts, Stijn Helsloot, Ivan Tsonev, Niek den Harder, Gerard van Rooij, Annemie Bogaerts

Role of volume and surface processes in the atomic oxygen loss frequency in oxygen glow discharges in Pyrex

This work aims at understanding and finding the most accurate way to estimate an effective O surface recombination probability from the temporal evolution of O(3P) density measured in modulated current conditions in the positive column of oxygen glow discharges in Pyrex, which is relevant for experimental characterization and for model inputs.
Authors: Pedro Viegas, Tiago Cunha Dias and Vasco Guerra

Non-thermal plasma assisted methane oxidation inside a DBD reactor: Effect of monometallic catalyst on energy efficiency and CO2 selectivity

The oxidation of methane was studied in a co-axial dielectric barrier discharge (DBD) quartz tube reactor at room temperature and atmospheric pressure.
Authors: Abhinash Kumar Singh, Jasmiina Palo, Johanna Kihlman, Tiina Heikola, Mika Suvanto, Pekka Simell, Niko M. Kinnunen

Trace Methane Destruction within the Effluent of Microwave Plasma

The authors experimentally investigated the use of microwave plasma to destroy trace methane (below 1 mol %) in a setup simulating cow barn emissions. A range of gases was evaluated in the plasma, and methane-containing air was injected downstream with the aim that excited species formed in the plasma would convert methane into valuable products and into species with a lower global warming potential, such as CO₂.
Authors: Stijn Helsloot, Omid Samadi, Muzammil Iqbal, Gerard van Rooij, Thomas Butterworth

Master’s Thesis: Combined non-thermal plasma and catalytic oxidation of low concentration methane

This master´s thesis by Irzam Javed studies the effect of non-thermal plasma and the hybridized plasma-catalysis system on the methane abatement by using Dielectric Barrier Discharge (DBD) reactor. The catalysts in the hybridized plasma-catalysis system are found to enhance the selectivity towards carbon dioxde..

Investigation of O atom kinetics in O2 plasma and its afterglow

This publication describes the development of a comprehensive kinetic model to study the O atom kinetics in an O2 plasma and its afterglow.
Authors: Matthias Albrechts, Ivan Tsonev and Annemie Bogaerts

Can post-plasma CH4 injection improve plasma-based dry reforming of methane? A modeling study

This study evaluates the energy efficiency and conversion performance of thermal plasma-driven dry reforming of methane using a pure CO₂ plasma with post-plasma CH₄ injection, supported by chemical kinetics modeling and comparison with classical DRM approaches.
Authors: Matthias Albrechts, Ivan Tsonev and Annemie Bogaerts

Deliverables

D2.1 – CHEMICAL KINETICS AND COMPUTATIONAL FLUID DYNAMICS MODEL

D2.4 – OXYGEN PRODUCTION EFFICIENCY AND CH4 REMOVAL EFFICIENCY IN MICROWAVE PLAMSA

D4.1 – TEST REPORT ON THE BARN AS OPERATIONAL ENVIRONMENT FOR METHANE ABATEMENT PROCESSES

D5.1 – AN OPERATIONAL MODEL OF THE BARN AND INTERNAL AIR QUALITY